活性物质
非平衡态热力学
润湿
流体力学
机械
化学物理
边界(拓扑)
软物质
乳状液
纳米技术
材料科学
物理
经典力学
化学
复合材料
热力学
生物
细胞生物学
数学分析
物理化学
胶体
生物化学
数学
作者
Raymond Adkins,Itamar Kolvin,Zhihong You,Sven Witthaus,M. Cristina Marchetti,Zvonimir Dogic
出处
期刊:Science
[American Association for the Advancement of Science]
日期:2022-08-11
卷期号:377 (6607): 768-772
被引量:52
标识
DOI:10.1126/science.abo5423
摘要
Controlling interfaces of phase-separating fluid mixtures is key to the creation of diverse functional soft materials. Traditionally, this is accomplished with surface-modifying chemical agents. Using experiment and theory, we studied how mechanical activity shapes soft interfaces that separate an active and a passive fluid. Chaotic flows in the active fluid give rise to giant interfacial fluctuations and noninertial propagating active waves. At high activities, stresses disrupt interface continuity and drive droplet generation, producing an emulsion-like active state composed of finite-sized droplets. When in contact with a solid boundary, active interfaces exhibit nonequilibrium wetting transitions, in which the fluid climbs the wall against gravity. These results demonstrate the promise of mechanically driven interfaces for creating a new class of soft active matter.
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