响应度
材料科学
光电探测器
光电子学
紫外线
响应时间
载流子
肖特基势垒
吸收(声学)
暗电流
肖特基二极管
氮化镓
上升时间
电子迁移率
纳米颗粒
氧化物
时滞与积分
电荷(物理)
瞬态响应
光学
氧化铝
镓
纳米技术
工作(物理)
肖特基效应
作者
Xiao-Dong Li,Zhiqing Tu,Nan Ding,Xiu Gong
摘要
ABSTRACT The inherent trade‐off between responsivity and response speed fundamentally limits the performance of solar‐blind ultraviolet photodetectors (SBUVPDs). Herein, an interfacial conductive‐bridge‐enhanced charge transport effect is proposed to overcome this limitation. Specifically, the 2D Nb 2 CT X MXene is introduced to form a charge transport channel at the surface of beta‐phase gallium oxide (β‐Ga 2 O 3 ). Aluminum (Al) nanoparticles (NPs) are incorporated as an efficient “carrier bridge” at the β‐Ga 2 O 3 /Nb 2 CT X MXene interface, effectively suppressing carrier accumulation and enhancing charge extraction. Meanwhile, decorating β‐Ga 2 O 3 with Al NPs enables a synergistic integration of plasmon‐enhanced light absorption and improved carrier dynamics via Schottky junction formation. Consequently, the β‐Ga 2 O 3 /Al NPs/Nb 2 CT X MXene SBUVPDs achieve remarkable performance, featuring a responsivity of 0.64 A/W, a detectivity of 1.01 × 10 13 Jones, a low dark current (8.94 × 10 −13 A), and a fast response time of 19.1 µs under 250 nm illumination. In addition, the responsivity of the SBUVPDs shows almost no degradation after 10 4 ON/OFF cycles. Finally, the device demonstrates excellent solar‐blind imaging capability for both static letters and real‐time moving objects. This work provides a novel and effective design strategy for next‐generation high‐performance SBUVPDs in imaging and sensing applications.
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