Novel Flexible Self-Standing Pt/Al2O3 Nanofibrous Membranes: Synthesis and Multifunctionality for Environmental Remediation

In spite of intensive research investigating the prevalent Pt/Al 2 O 3 catalysts, achieving macroscopic morphology beyond the powder form limitations remains highly challenging. Meanwhile, current impregnation-based preparation approaches show the drawbacks of tedious procedures and inefficient use of noble metals. Therefore, it is important to search for new methods for the fabrication of Pt/Al 2 O 3 catalysts with a novel morphology. In this study, a novel Pt/Al 2 O 3 nanofibrous membrane catalyst is fabricated via a facile one-pot electrospinning process. The embedding of Pt nanoparticles is performed simultaneously with the formation of Al 2 O 3 nanofibers. The Pt/Al 2 O 3 membranes show remarkable mechanical properties with tensile stresses as high as 44.14 MPa. Notably, the Pt/Al 2 O 3 membranes exhibit multifunctionality with excellent performance characteristics. The catalytic experiments indicate that 100% of bisphenol A is removed within 60 min, and 100% of CO is completely converted to CO 2 at 242 °C when Pt/Al 2 O 3 membranes are used as catalysts. The membranes also exhibit excellent filtration performance, clearly decreasing the turbidity of water, and meet the high efficiency of particulate air filter standards. The excellent flexibility, satisfying mechanical property, and multifunctionality extend the range of potential application of the Pt/Al 2 O 3 membranes. Moreover, the facile synthesis suggests new possibilities for the fabrication of many membrane-form Al 2 O 3 -supported catalysts.