环境友好型
超声
涂层
木质素
接触角
材料科学
制作
聚合物
纳米技术
溶剂
光热治疗
化学工程
复合材料
化学
有机化学
工程类
病理
生物
替代医学
医学
生态学
作者
Bole Ma,Fuquan Xiong,Hang Wang,Yan Qing,Fuxiang Chu,Yiqiang Wu
标识
DOI:10.1016/j.cej.2023.141309
摘要
Exploring the tailorable and scalable production method of lignin micro-nanospheres (LMNS) have a significant meaning for expanding their application field. In this study, the fabrication of LMNS with a wide size-controlled range (∼30 nm to ∼3 μm) and high solid content (8 mg mL−1) by dynamics regulation in a γ-valerolactone/water binary system was reported. The LMNS could be controllably fabricated from nano to micron-scale by synergistically regulating four main dynamics factors, i.e., initial lignin concentration, lignin solution/water ratio, temperature of lignin solution and water, and sonication time. Moreover, the uniformity of the LMNS was effectively improved by centrifugation. The as-fabricated LMNS were further used to fabricate functional superhydrophobic coating on the surface of wood, with a water contact angle of 164.4° and a sliding angle of 5°. The coating showed excellent mechanical and chemical stability in a series of tests, especially good resistance to organic solvent. The coating also exhibited great photothermal effect, suggesting potential application in high-efficient deicing and antibacterial. This study not only provides a green and effective strategy for tailorable and scalable production of LMNS, but also presents an innovative concept for LMNS to fabricate the functional superhydrophobic coatings with organic solvent resistance and photothermal effect.
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