Strengthening the Metal–Acid Interactions by Using CeO2 as Regulators of Precisely Placing Pt Species in ZSM‐5 for Furfural Hydrogenation

@ZSM-5 catalyst possesses remarkably-improved activity and selectivity, which can convert >99% furfural into cyclopentanone with 97.2% selectivity in 6 h at 160 °C. Besides the excellent catalytic performance, the ordered metal-acid distribution also makes such kind of catalyst an ideal research subject for metal-acid interactions. The following mechanization investigation reveals that the enhancement is strongly related to the unique encapsulation structure, which promotes the migration of the reactants over different active sites, thereby contributing to the tandem reaction.