异质结
材料科学
纳米复合材料
纳米结构
热液循环
纳米技术
吸附
密度泛函理论
化学工程
光电子学
化学
工程类
计算化学
有机化学
作者
Qui Thanh Hoai Ta,Nguyen Ngoc Tri,Jin‐Seo Noh
标识
DOI:10.1016/j.apsusc.2022.154624
摘要
In this study, novel MoS2/Ti3C2Tx heterostructures were prepared from Ti3C2Tx MXene via a hydrothermal strategy. The well-bonded interface developed between the MoS2 nanostructure and the conductive Ti3C2Tx MXene played a crucial role in improving the sensing abilities of the prepared heterostructures compared to their pristine counterparts. Owing to the synergistic interplay effect, the optimal MoS2/Ti3C2Tx heterostructure exhibited room-temperature NO2 sensing activity with a rapid response and full recovery at low gas concentrations. To understand the high sensitivity, density functional theory calculations were used to observe stable configurations and adsorption behaviors. The proposed concept may provide an archetype for understanding the sensing characteristics of materials for NO2 detection at room temperatures.
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