甲酰胺
甲醇
法拉第效率
电合成
电化学
氨
氮气
氨生产
选择性
化学
电催化剂
无机化学
材料科学
化学工程
催化作用
有机化学
电极
物理化学
工程类
作者
Nannan Meng,Jiang Shao,Hongjiao Li,Yuting Wang,Fu Xiaoli,Cuibo Liu,Yifu Yu,Bin Zhang
标识
DOI:10.1038/s41467-022-33232-w
摘要
Electrochemical conversion of abundant carbon- and nitrogen-containing small molecules into high-valued organonitrogen compounds is alluring to reducing current dependence on fossil energy. Here we report a single-cell electrochemical oxidation approach to transform methanol and ammonia into formamide under ambient conditions over Pt electrocatalyst that provides 74.26% selectivity from methanol to formamide and a Faradaic efficiency of 40.39% at 100 mA cm
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