Rational design of two-dimensional architectures for efficient electrocatalysis

In this thesis, the principal focus is the rational design and fabrication of two-dimensional (2D) nanoarchitectures, e.g., low-cost metal oxide nanosheets and earth-abundant transition metal layered double hydroxides (LDHs) for enhanced electrocatalysis. The related hydrogen evolution reaction (HER) and oxygen evolution reaction (OER) performance not only demonstrated the advances of 2D nanomaterials, such as unique physical and mechanical properties, unprecedented electronic features, and ultrahigh surface areas but also indicated the possible mechanisms behind boosted activity and stability, e.g., phase engineering function and oxygen vacancies influence.