Efficient Second-Harmonic Generation in Thin-Film Lithium Tantalate Through Modal Phase-Matching

Lithium tantalate (LT) exhibits nonlinear optical properties that are comparable to those of lithium niobate (LN), yet the former surpasses the latter in several respects. These include an enhanced optical damage threshold, a wider transparency range, and lower birefringence. Consequently, LT is an excellent material for optical frequency conversion applications. In this study, we have devised a novel device based on thin-film lithium tantalate (TFLT) for the efficient generation of second-harmonic waves. The design employs modal phase-matching (MPM), which circumvents the intricacies of conventional poling techniques, and attains a normalised conversion efficiency of 120% W−1cm−2. In order to address the challenges presented by higher-order modes, a mode converter with an insertion loss of less than 0.1 dB has been developed, thereby ensuring the efficient utilisation of the second harmonic. This study not only demonstrates the potential of TFLT for high-performance SHG, but also promotes the development of integrated nonlinear TFLT platforms.