光催化
异质结
材料科学
无定形固体
化学工程
碳纤维
无定形碳
碳膜
纳米技术
化学
薄膜
光电子学
复合材料
催化作用
复合数
有机化学
工程类
作者
Yu Sun,Yanling Yang,Huajun Chen,Jiajun Liu,Xiao‐Lei Shi,Guoquan Suo,Xiaojiang Hou,Xiaohui Ye,Li Zhang,Siyu Lu,Zhi‐Gang Chen
标识
DOI:10.1016/j.jcis.2023.07.177
摘要
Most traditional powder photocatalysts are not easily recovered. Herein, we report a flexible and recoverable photocatalyst with superior photocatalytic activity, in which MoS2/TiO2 heterojunctions are grown on amorphous carbon-coated carbon textiles (CT@C-MoS2/TiO2). Recoverable CT@C-MoS2/TiO2 textile was used to degrade 10 mg L-1 rhodamine B, leading to a degradation rate of up to 98.8 % within 30 min. Such a degradation rate is much higher than that of most of the reported studies. A density functional theory (DFT) calculation results illustrate charge transfer mechanism inside TiO2-C, MoS2-C, and MoS2/TiO2 heterojunctions, which shows that CT@C-MoS2/TiO2 textile with three electron separation channels has a high photogenerated carrier separation rate, which remarkably enhances the photocatalytic activity. Our work provides a novel strategy to design an efficient and recoverable photocatalyst with high activity.
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