Bidirectional Vectorial Holography Using Bi‐Layer Metasurfaces and Its Application to Optical Encryption

Abstract The field of optical systems with asymmetric responses has grown significantly due to their various potential applications. Janus metasurfaces are noteworthy for their ability to control light asymmetrically at the pixel level within thin films. However, previous demonstrations are restricted to the partial control of asymmetric transmission for a limited set of input polarizations, focusing primarily on scalar functionalities. Here, optical bi‐layer metasurfaces that achieve a fully generalized form of asymmetric transmission for any input polarization are presented. The designs owe much to the theoretical model of asymmetric transmission in reciprocal systems, which elucidates the relationship between front‐ and back‐side Jones matrices in general cases. This model reveals a fundamental correlation between the polarization‐direction channels of opposing sides. To circumvent this constraint, partitioning the transmission space is utilized to realize four distinct vector functionalities within the target volume. As a proof of concept, polarization‐direction‐multiplexed Janus vectorial holograms generating four vectorial holographic images are experimentally demonstrated. When integrated with computational vector polarizer arrays, this approach enables optical encryption with a high level of obscurity. The proposed mathematical framework and novel material systems for generalized asymmetric transmission may pave the way for applications such as optical computation, sensing, and imaging.