激光阈值
纳米线
卤化物
激光器
材料科学
钙钛矿(结构)
光电子学
铯
纳米尺度
激发
纳米技术
光学
化学
电气工程
无机化学
波长
物理
工程类
结晶学
作者
Samuel W. Eaton,Minliang Lai,Natalie A. Gibson,Andrew Barnabas Wong,Letian Dou,Jie Ma,Lin‐Wang Wang,Stephen R. Leone,Peidong Yang
标识
DOI:10.1073/pnas.1600789113
摘要
The rapidly growing field of nanoscale lasers can be advanced through the discovery of new, tunable light sources. The emission wavelength tunability demonstrated in perovskite materials is an attractive property for nanoscale lasers. Whereas organic-inorganic lead halide perovskite materials are known for their instability, cesium lead halides offer a robust alternative without sacrificing emission tunability or ease of synthesis. Here, we report the low-temperature, solution-phase growth of cesium lead halide nanowires exhibiting low-threshold lasing and high stability. The as-grown nanowires are single crystalline with well-formed facets, and act as high-quality laser cavities. The nanowires display excellent stability while stored and handled under ambient conditions over the course of weeks. Upon optical excitation, Fabry-Pérot lasing occurs in CsPbBr3 nanowires with an onset of 5 μJ cm(-2) with the nanowire cavity displaying a maximum quality factor of 1,009 ± 5. Lasing under constant, pulsed excitation can be maintained for over 1 h, the equivalent of 10(9) excitation cycles, and lasing persists upon exposure to ambient atmosphere. Wavelength tunability in the green and blue regions of the spectrum in conjunction with excellent stability makes these nanowire lasers attractive for device fabrication.
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