材料科学
发光二极管
光电子学
纳米晶
量子效率
发光效率
二极管
各向异性
亮度
固态照明
基质(水族馆)
电致发光
纳米技术
光学
图层(电子)
物理
海洋学
地质学
作者
Yunke Zhu,Yunzhou Deng,Peng Bai,Xiang Wu,Yige Yao,Qinyun Liu,Jingjing Qiu,Hu Ai,Zhenyu Tang,Wenjin Yu,Pengzuo Jiang,Yaolong Li,Zhetong Liu,Peng Gao,Yanlei Hao,Wangxiao Jin,Desui Chen,Xingyi Zhu,Yizheng Jin,Yunan Gao
标识
DOI:10.1002/adma.202305382
摘要
Nanocrystal-based light-emitting diodes (Nc-LEDs) have immense potential for next-generation high-definition displays and lighting applications. They offer numerous advantages, such as low cost, high luminous efficiency, narrow emission, and long lifetime. However, the external quantum efficiency (EQE) of Nc-LEDs, typically employing isotropic nanocrystals, is limited by the out-coupling factor. Here efficient, bright, and long lifetime red Nc-LEDs based on anisotropic nanocrystals of colloidal quantum wells (CQWs) are demonstrated. Through modification of the substrate's surface properties and control of the interactions among CQWs, a self-assembled layer with an exceptionally high distribution of in-plane transitions dipole moment of 95%, resulting in an out-coupling factor of 37% is successfully spin-coated. The devices exhibit a remarkable peak EQE of 26.9%, accompanied by a maximum brightness of 55 754 cd m-2 and a long operational lifetime (T95 @100 cd m-2 ) over 15 000 h. These achievements represent a significant advancement compared to previous studies on Nc-LEDs incorporating anisotropic nanocrystals. The work is expected to provide a general self-assembly strategy for enhancing the light extraction efficiency of Nc-LEDs based on anisotropic nanocrystals.
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