膜
材料科学
拉曼光谱
光电子学
热导率
光子学
表征(材料科学)
堆栈(抽象数据类型)
光致发光
纤锌矿晶体结构
热的
光谱学
半导体
热分析
量子阱
外延
量子点
热阻
光子晶体
纳米技术
光学
作者
Wilken Seemann,Mahmoud Elhajhasan,Julian Themann,Katharina Dudde,Guillaume Würsch,Jana Lierath,Gordon Callsen,Joachim Ciers,Åsa Haglund,Nakib H. Protik,Giuseppe Romano,R. Butté,Jean-François Carlin,N. Grandjean
摘要
Semiconductor membranes are widely used in research fields that target medical, biological, environmental, and optical applications. Often such membranes derive their functionality from a nanopatterning, which challenges the determination of their optical, electronic, mechanical, and thermal properties. In this work, we demonstrate the noninvasive, all-optical thermal characterization of approximately-800-nm-thick and approximately-150- μ m -wide membranes that consist mainly of wurtzite GaN and a stack of In 0.15 Ga 0.85 N quantum wells as a built-in light source. Because of their application in photonics, e.g., for vertical-cavity surface-emitting lasers, such photonic membranes are bright light emitters, which challenges their thermal characterization by optical means. We combine top-view two-laser Raman thermometry (2LRT) with time-resolved photoluminescence spectroscopy to extract the in-plane thermal conductivity κ in~plane of these membranes, which represents a notable difference from previous studies on epitaxial GaN films. Thus, we can disentangle the entire laser-induced power balance. Thermal imaging by Raman spectroscopy yields κ in plane = 165 − 14 + 16 W m − 1 K − 1 for the best membrane. This result compares well with κ in plane = 177 W m − 1 K − 1 obtained by simulations based on a solution of the linearized phonon Boltzmann transport equation, including three- and four-phonon scattering, as well as phonon-isotope and phonon-boundary scattering. Furthermore, we study how κ in plane is affected by a roughening of the membrane’s back side and additional semiconductor layers. For the membrane with the roughest back side, we observe a reduction of κ in plane by almost 40%, which is accompanied by an anisotropy of κ in plane due to etch channel formation. Thanks to the 2LRT approach, such variations and anisotropies of κ in plane become accessible to the experimentalist via highly spatially resolved temperature maps.
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