吸附
介孔材料
选择性
超声
废水
石墨烯
氧化物
化学工程
单层
可重用性
核化学
化学
无机化学
材料科学
有机化学
色谱法
纳米技术
催化作用
废物管理
生物化学
工程类
计算机科学
程序设计语言
软件
作者
Changlong Bi,Chunhong Zhang,Fuqiu Ma,Xu Zhang,Ming Yang,Jinru Nian,Lijia Liu,Hongbiao Dong,Lien Zhu,Qiang Wang,Shixi Guo,Qingtao Lv
标识
DOI:10.1016/j.micromeso.2021.111223
摘要
In this study, a mesoporous PCN-222/GO-COOH adsorbent, based on the growth of a mesoporous zirconium-metalloporphyrin metal-organic framework (PCN-222) on the carboxylated graphene oxide (GO-COOH) to recover U(VI) from wastewater, was designed and prepared through solvothermal method and ultrasonication assisted stir technique. The U(VI) adsorption performance of the PCN-222/GO-COOH adsorbent was evaluated. The results indicated that the mesoporous PCN-222/GO-COOH adsorbent could effectively recover U(VI) and show an excellent adsorption capacity (426 mg/g), which was superior to those of GO-COOH and PCN-222 probably because the complexation and synergistic effect between GO-COOH and PCN-222 were facilitated by the ultrasonication assisted stir technique. And the PCN-222/GO-COOH adsorbent showed excellent reusability and selectivity for U(VI) adsorption, which also had outstanding adsorption performances in the complex wastewater. Furthermore, the chemical and monolayer adsorption dominated the U(VI) adsorption behavior of PCN-222/GO-COOH adsorbent. The excellent adsorption capacity, selectivity and reusability for U(VI) rendered PCN-222/GO-COOH composites as a promising adsorbent for recovering U(VI) from wastewater.
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