Light‐Induced Electric Field Enhanced Self‐Powered Photodetector Based on Van der Waals Heterojunctions

Self-powered photodetectors have attracted widespread attention due to their low power consumption which can be driven by the built-in electric field instead of external power, but it is very difficult to achieve high responsivity and fast response speed concurrently. Here, a self-powered photodetector with light-induced electric field enhancement based on a 2D InSe/WSe₂ /SnS₂ van der Waals heterojunction is designed. The light-induced electric field derived from the photo-generated electrons of SnS₂ accumulated at the SnS₂ /WSe₂ interface produces an additional negative gate voltage applied to the WSe₂ layer, which enhances the built-in electric field in the InSe/WSe₂ /SnS₂ heterojunction. Accordingly, the photocurrent and photoresponse speed of the heterostructure device are largely improved. The self-powered photodetector based on the InSe/WSe₂ /SnS₂ heterostructure exhibits a high responsivity of 550 mA W^-1 , which is a 50 times increase compared to the InSe/WSe₂ photodetector, and the response speed (110/120 µs) is one order of magnitude faster than that of the InSe/WSe₂ photodetector. The high responsivity and fast speed are caused by the stronger built-in electric field modulated by a light-induced electric field, which can separate carriers effectively and reduce drift times. This device architecture can provide a new avenue to fabricate high-responsivity, fast self-power photodetectors by utilizing the van der Waals heterojunction.