甲醛
光催化
纳米复合材料
辐照
光化学
降级(电信)
产量(工程)
材料科学
化学工程
化学
催化作用
纳米技术
有机化学
复合材料
物理
工程类
计算机科学
核物理学
电信
作者
Xi Rao,Hailong Dou,Dan Long,Yongping Zhang
出处
期刊:Chemosphere
[Elsevier]
日期:2020-04-01
卷期号:244: 125462-125462
被引量:26
标识
DOI:10.1016/j.chemosphere.2019.125462
摘要
A series of Ag3PO4/g-C3N4 nanocomposites were synthesized by introducing various small amount of Ag3PO4 in g-C3N4 and subsequently employed for decomposing formaldehyde (HCHO) in continuous flow as photocatalysts. The results show that all the Ag3PO4/g-C3N4 nanocomposites could perform a very stable photoactivity for degrading continuously flowing gaseous formaldehyde for at least 600 h. Especially, the HCHO degradation rate reached 22.4% by using 1AP-CN, which was 2.63 times as fast as that of g-C3N4. Our results reveal that the photoinduced electrons in conduction band (CB) are trapped by O2 to yield ⋅O2−, while holes in valence band (VB) directly oxidize –OH and/or water to produce ·OH under visible light irradiation. As a consequence, HCHO is further oxidized to CO2 and H2O by as-generate active species.
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