石墨氮化碳
光催化
氮化碳
过氧化氢
催化作用
制氢
材料科学
纳米技术
碳纤维
氧化还原
吸附
载流子
选择性
化学
化学工程
无机化学
有机化学
复合数
工程类
复合材料
光电子学
作者
Chao Liang,Xuemin Wang,Wei Liu,Huiyun Liu,Da-Wei Huang,Yuanzheng Zhang,Kai-Hang Zhang,Lisha Jiang,Yu-Yu Jia,Cheng-Gang Niu
标识
DOI:10.1016/j.cej.2023.142931
摘要
Hydrogen peroxide (H2O2) is a crucial chemical compound for numerous applications in industrial processes, medical disinfection, and water treatment. Graphitic carbon nitride (g-C3N4) is a promising alternative for photocatalytic H2O2 production, thanks to its high redox ability, long term-stability, and adjustable electronic properties. However, the photocatalytic H2O2 production in g-C3N4-based systems is typically limited by sluggish kinetics, rapid charge carrier recombination, and low H2O2 production selectivity. To address these issues, functionalized g-C3N4 materials with a large surface area, fast charge carrier separation, and improved O2 adsorption and activation are expected to enhance reaction kinetics and enhance H2O2 production selectivity. In this review, we introduce the fundamental principles of photocatalytic H2O2 production and summarize the recent progress in g-C3N4-based materials for photocatalytic H2O2 production. We also briefly discuss applications of photocatalytic H2O2 production and provide insights into the existing challenges and meaningful perspectives of g-C3N4 to advance the growing field of H2O2 production.
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