价(化学)
磁性
材料科学
铁磁性
凝聚态物理
晶体结构
旋转
结晶学
物理
化学
量子力学
作者
Greeshma C. Jose,Kaleb Burrage,J. Jimenez,Weiwei Xie,Barbara Lavina,Jiyong Zhao,E. Ercan,Dongzhou Zhang,Yuming Xiao,Yogesh K. Vohra,Wenli Bi
出处
期刊:Physical review
[American Physical Society]
日期:2023-06-12
卷期号:107 (24)
被引量:8
标识
DOI:10.1103/physrevb.107.245121
摘要
${\mathrm{EuCd}}_{2}{\mathrm{As}}_{2}$ has been proposed to be one of the ideal platforms as an intrinsic topological magnetic system, potentially hosting a single pair of Weyl points when it is tuned into the ferromagnetic state with spins aligned out of plane by either external pressure or chemical doping. To investigate the possible realization of an ideal topological state, we have systematically investigated pressure control of the magnetic state, valence, and crystal structure using synchrotron-based time-domain M\"ossbauer spectroscopy, x-ray absorption spectroscopy, and powder x-ray diffraction. Our experimental results show that the magnetic configuration remains mostly in plane under pressure up to 42.8 GPa and pressure effectively enhances the magnetic ordering temperature. Meanwhile, Eu ions remain divalent when subjected to pressure up to 35.9 GPa, and the trigonal crystal lattice is maintained up to 34.6 GPa. Our work provides valuable experimental data to benchmark future theoretical studies in magnetic topological materials.
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