声子
黛比
凝聚态物理
各向同性
德拜模型
无定形固体
物理
分子振动
离域电子
瑞利散射
弹性(物理)
玻色子
衰减
散射
材料科学
量子力学
热力学
结晶学
化学
分子
作者
Shivam Mahajan,Massimo Pica Ciamarra
标识
DOI:10.1103/physrevlett.127.215504
摘要
The vibrational density of states D(ω) of solids controls their thermal and transport properties. In crystals, the low-frequency modes are extended phonons distributed in frequency according to Debye's law, D(ω)∝ω^{2}. In amorphous solids, phonons are damped, and at low frequency D(ω) comprises extended modes in excess over Debye's prediction, leading to the so-called boson peak in D(ω)/ω^{2} at ω_{bp}, and quasilocalized ones. Here we show that boson peak and phonon attenuation in the Rayleigh scattering regime are related, as suggested by correlated fluctuating elasticity theory, and that amorphous materials can be described as homogeneous isotropic elastic media punctuated by quasilocalized modes acting as elastic heterogeneities. Our numerical results resolve the conflict between theoretical approaches attributing amorphous solids' vibrational anomalies to elastic disorder and localized defects.
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