光伏系统
卤化物
钙钛矿(结构)
替代(逻辑)
太阳能电池
材料科学
光电子学
化学工程
Mercury(编程语言)
无机化学
化学
结晶学
计算机科学
生物
工程类
程序设计语言
生态学
作者
Pavel A. Troshin,Denis V. Anokhin,Kirill L. Gerasimov,Nadezhda N. Dremova,Pavel A. Troshin
标识
DOI:10.1021/acs.jpclett.6b02122
摘要
Here we report a systematic study of the Pb2+ substitution in the hybrid iodoplumbate MAPbI3 with a series of elements affecting optoelectronic, structural, and morphological properties of the system. It has been shown that even partial replacement of lead with Cd2+, Zn2+, Fe2+, Ni2+, Co2+, In3+, Bi3+, Sn4+, and Ti4+ results in a significant deterioration of the photovoltaic characteristics. On the contrary, Hg-containing hybrid MAPb1-xHgxI3 salts demonstrated a considerably improved solar cell performance at optimal mercury loading. This result opens up additional dimension in the compositional engineering of the complex lead halides for designing novel photoactive materials with advanced optoelectronic and photovoltaic properties.
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