丙酮
材料科学
纳米片
热液循环
选择性
微观结构
复合材料
化学工程
纳米技术
化学
有机化学
工程类
催化作用
作者
Miao Liu,Jun Ji,Peng Song,Min Liu,Qi Wang
标识
DOI:10.1016/j.snb.2021.130782
摘要
MXene combining with metal oxide semiconductor (MOS) can improve carrier transfer rate, inhibit agglomeration, and promote the improvement of gas-sensing performance. In this article, the heterogeneous composites of α-Fe2O3 and Ti3C2Tx MXene were successfully synthesized through a facile hydrothermal route, and characterized the morphology and microstructure by various characterizations. The results revealed that the α-Fe2O3 nanocubes with sizes of around 250 nm in width were prepared and uniformly distributed to the surface of the Ti3C2Tx MXene nanosheet. Gas-sensing test results illustrated that the α-Fe2O3/Ti3C2Tx MXene composites-based sensor exhibited outstanding selectivity to acetone compared with other typical gases, and illustrated a high response (16.6% to 5 ppm acetone), the fast response and recovery speeds (5/5 s), superb linearity and prominent repeatability at room temperature (RT). Furthermore, the gas-sensing mechanism of the α-Fe2O3/Ti3C2Tx MXene sensor toward acetone is discussed by density functional theory (DFT) calculation. This work is expected to provide useful reference to develop other promising hybrids for acetone sensing at RT.
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