Morphology-Controlled Transition between Interfacial Slip and Drag over a Pinned Surface Nanobubble under Electrowetting-Inspired Control

阻力 打滑(空气动力学) 润湿 材料科学 机械 剪切(地质) 气泡 非平衡态热力学 剪切流 流量(数学) 接触角 复合材料 分子动力学 变形(气象学) 纳米技术 边值问题 凝聚态物理 剪切速率 固体表面 剪应力 经典力学 身体力量
作者
Yan Chen,Yunyun Zhang,Xiaolong Zhang,Chong Qiao
出处
期刊:Langmuir [American Chemical Society]
标识
DOI:10.1021/acs.langmuir.6c01587
摘要

Abstract Surface nanobubbles are known to influence interfacial slip and near-wall hydrodynamics, yet the role of actively controlled nanobubble morphology in regulating momentum transfer at solid–liquid interfaces remains insufficiently understood. Here, nonequilibrium molecular dynamics simulations are used to investigate a pinned surface nanobubble located at a wettability step in a confined water nanochannel. An electrowetting-inspired interfacial forcing (Fext) is applied near the solid surface to tune the effective solid–liquid wettability, thereby inducing reversible deformation of the pinned nanobubble from a flattened configuration to a more protruding morphology. The resulting velocity fields, effective slip lengths, and wall shear stresses reveal a pronounced nonmonotonic dependence of hydrodynamic drag on nanobubble morphology. For small protrusion angles, the gas–liquid interface behaves as a slip boundary that reduces near-wall viscous dissipation. As the protrusion angle increases, the nanobubble increasingly acts as a geometric obstacle, inducing flow recirculation and increasing flow resistance. Bubble deformation is also accompanied by internal gas-phase circulation that couples with the external shear flow and modifies the near-wall hydrodynamics. These results clarify how nanobubble morphology mediates the transition between slip enhancement and drag increase and provide insight into flow regulation at gas-structured interfaces.
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