油页岩
溶解
吸附
提高采收率
石油工程
基质(化学分析)
固碳
碳酸盐
化学工程
页岩油
水银孔隙仪
碳氢化合物
地质学
萃取(化学)
环境科学
多孔性
矿物学
化学
多孔介质
吸附
二氧化碳
岩土工程
色谱法
有机化学
工程类
古生物学
作者
Angela Goodman,Sean Sanguinito,Barbara Kutchko,Sittichai Natesakhawat,Patricia Cvetic,Andrew J. Allen
出处
期刊:Fuel
[Elsevier]
日期:2020-04-01
卷期号:265: 116930-116930
被引量:53
标识
DOI:10.1016/j.fuel.2019.116930
摘要
Shale unconventional reservoirs are currently and expected to remain substantial fossil fuel resources in the future. As CO2 is being considered to enhance oil recovery and for storage purposes in unconventional reservoirs, it is unclear how the shale matrix and fractures will react with CO2 and water during these efforts. Here, we examined the Utica Shale and its reactivity with CO2 and water using scanning electron microscopy, N2 and CO2 sorption isotherms, mercury intrusion porosimetry, and X-ray scattering methods. During CO2 exposure, the presence of water can inhibit CO2 migration into the shale matrix, promote carbonate dissolution, and dramatically change the pore scale variability by opening and closing pore networks over the macro- to nano-scale range. These alterations in the shale matrix could impact flow pathways and ultimately, oil recovery factors and carbon storage potential.
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