Sunflower-Stalk-Based Solar-Driven Evaporator with a Confined 2D Water Channel and an Enclosed Thermal-Insulating Cellular Structure for Stable and Efficient Steam Generation

材料科学 海水淡化 蒸发器 低温热脱盐 蒸发 太阳能淡化 化学工程 纳米技术 热交换器 机械工程 化学 生物化学 热力学 物理 工程类
作者
Fangqingxin Liu,Linmin Xia,Lingyan Zhang,Fei Guo,Xuexia Zhang,Yan Yu,Rilong Yang
出处
期刊:ACS Applied Materials & Interfaces [American Chemical Society]
卷期号:13 (46): 55299-55306 被引量:38
标识
DOI:10.1021/acsami.1c20747
摘要

Given the worsening freshwater scarcity around the world, the interfacial solar-driven steam generation for seawater desalination and wastewater treatment has attracted wide attention due to its rich energy resources, convenience, and environmental friendliness. However, challenges still remain for developing high-efficiency interfacial solar-driven steam generation devices from low-cost, readily available, and green material resources. Herein, taking advantage of the delicate composite structure of the sunflower stalk, a sunflower-stalk-based solar-driven evaporator with a confined two-dimensional (2D) water supply pathway and an enclosed thermal-insulating structure is reported. The pith of sunflower stalks is composed of well-arranged honeycomb-like parenchyma cells that endow sunflower stalks with low thermal conductivity comparable to that of synthetic plastic foam. The low-tortuosity vascular bundles in the skin can serve as a natural 2D water pathway for rapid water transportation. The benefit of these functions is that an evaporator based on a carbon-nanotube-coated sunflower stalk (C-Ss) achieves a high evaporation rate of 1.76 kg m-2 h-1 under 1 sun irradiation (1 kW m-2). The C-Ss also shows a highly stable evaporation performance, high ion rejection efficiency, and a self-cleaning ability during the actual seawater desalination process. With advantages of abundant resources, easy fabrication, and sustainability, this C-Ss-based evaporator provides a promising choice for freshwater production in developing regions.
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