材料科学
纳米复合材料
纳米颗粒
相对湿度
异质结
苯胺
化学工程
聚合
湿度
肿胀 的
氨
响应时间
纳米技术
复合材料
聚合物
光电子学
有机化学
热力学
计算机图形学(图像)
工程类
物理
化学
计算机科学
作者
Lingling Wang,Hui Huang,Songhua Xiao,Daoping Cai,Yuan Liu,Bin Liu,Dandan Wang,Chenxia Wang,Liang Han,Yanrong Wang,Qiuhong Li,Taihong Wang
摘要
We report a room-temperature NH3 gas sensor with high response and great long-term stability, including CeO2 NPs conformally coated by cross-linked PANI hydrogel. Such core-shell nanocomposites were prepared by in situ polymerization with different weight ratios of CeO2 NPs and aniline. At room temperature, the nanohybrids showed enhanced response (6.5 to 50 ppm of NH3), which could be attributed to p-n junctions formed by the intimate contact between these two materials. Moreover, the stability was discussed in terms of phytic acid working as a gelator, which helped the PANI sheath accommodate itself and enhance the mechanical strength and chemical stability of the sensors by avoiding "swelling effect" in high relative humidity. The sensors maintained its sensing characteristic (response of ca. 6.5 to 50 ppm of NH3) in 15 days. Herein, the obtained results could help to accelerate the development of ammonia gas sensor.
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