甲酸
碳中和
催化作用
甲醇
碳纤维
温室气体
化石燃料
氢
转移加氢
纳米技术
材料科学
化学
生化工程
工艺工程
有机化学
工程类
生态学
生物
钌
复合材料
复合数
作者
Guangyu Chen,Jun Ma,Wanbing Gong,Jiayi Li,Zheyue Li,Ran Long,Yujie Xiong
出处
期刊:Nanoscale
[The Royal Society of Chemistry]
日期:2024-01-01
摘要
Under the background of carbon neutrality, the direct conversion of greenhouse CO2 to high value added fuels and chemicals is becoming an important and promising technology. Among them, the generation of liquid C1 products (formic acid and methanol) has made great progress; nevertheless, it encounters the problem of how to use it efficiently to solve the overcapacity issue. In this review, we suggest that the catalytic transfer hydrogenation using formic acid and methanol as the hydrogen sources is a critical and potential route for the substitution for the fossil fuel-derived H2 to generate essential bulk and fine chemicals. We mainly focus on summarizing the recent progress of heterogeneous catalysts in such reactions, including thermal- and photo-catalytic processes. Finally, we also propose some challenges and opportunities for this development.
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