Methane, Carbon Dioxide, and Nitrous Oxide Emissions from Septic Tank Systems

一氧化二氮 甲烷 二氧化碳 环境科学 温室气体 废物管理 化粪池 环境工程 化学 工程类 地质学 海洋学 有机化学
作者
Libia R. Diaz-Valbuena,Harold Leverenz,Christopher D. Cappa,George Tchobanoglous,William R. Horwáth,Jeannie L. Darby
出处
期刊:Environmental Science & Technology [American Chemical Society]
卷期号:45 (7): 2741-2747 被引量:100
标识
DOI:10.1021/es1036095
摘要

Emissions of CH4, CO2, and N2O from conventional septic tank systems are known to occur, but there is a dearth of information as to the extent. Mass emission rates of CH4, CO2, and N2O, as measured with a modified flux chamber approach in eight septic tank systems, were determined to be 11, 33.3, and 0.005 g capita(-1) day(-1), respectively, in this research. Existing greenhouse gas (GHG) emission models based on BOD (biochemical oxygen demand) loading have estimated methane emissions to be as high as 27.1 g CH4 capita(-1) day(-1), more than twice the value measured in our study, and concluded that septic tanks are potentially significant sources of GHGs due to the large number of systems currently in use. Based on the measured CH4 emission value, a revised CH4 conversion factor of 0.22 (compared to 0.5) for use in the emissions models is suggested. Emission rates of CH4, CO2, and N2O were also determined from measurements of gas concentrations and flow rates in the septic vent system and were found to be 10.7, 335, and 0.2 g capita(-1)day(-1), respectively. The excellent agreement in the CH4 emission rates between the flux chamber and the vent values indicates the dominant CH4 source is the septic tank.
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