量子点
电致发光
光电子学
红外线的
二极管
发光二极管
钙钛矿(结构)
发光
光致发光
材料科学
纳米技术
光子学
物理
光学
化学
结晶学
图层(电子)
作者
Xiwen Gong,Zhenyu Yang,Grant Walters,Riccardo Comin,Zhijun Ning,Eric M. Beauregard,Valerio Adinolfi,Oleksandr Voznyy,Edward H. Sargent
出处
期刊:Nature Photonics
[Nature Portfolio]
日期:2016-02-22
卷期号:10 (4): 253-257
被引量:413
标识
DOI:10.1038/nphoton.2016.11
摘要
Embedding quantum dots in a perovskite matrix yields efficient light emitters. Colloidal quantum dots (CQDs) are emerging as promising materials for constructing infrared sources in view of their tunable luminescence, high quantum efficiency and compatibility with solution processing1. However, CQD films available today suffer from a compromise between luminescence efficiency and charge transport, and this leads to unacceptably high power consumption. Here, we overcome this issue by embedding CQDs in a high-mobility hybrid perovskite matrix. The new composite enhances radiative recombination in the dots by preventing transport-assisted trapping losses; yet does so without increasing the turn-on voltage. Through compositional engineering of the mixed halide matrix, we achieve a record electroluminescence power conversion efficiency of 4.9%. This surpasses the performance of previously reported CQD near-infrared devices two-fold, indicating great potential for this hybrid QD-in-perovskite approach.
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