光催化
苯酚
可见光谱
水溶液
碳纤维
催化作用
石墨氮化碳
氮化碳
化学
氮化物
介孔材料
核化学
光化学
材料科学
无机化学
有机化学
图层(电子)
复合材料
复合数
光电子学
作者
Fenghui Liu,Jie Yu,Guangyuan Tu,Lijun Qu,Jin-Fen Xiao,Yongdi Liu,Lingzhi Wang,Juying Lei,Jinlong Zhang
标识
DOI:10.1016/j.apcatb.2016.08.001
摘要
In this study, carbon nitride was loaded into the titanium incorporated SBA-15 mesoporous silica (denoted as Ti-SBA15-CN) by a two-step vapor condensation of dicyandiamide. The as-prepared sample was characterized by various spectroscopy techniques. Photocatalytic reduction of Cr (VI) in aqueous solution was investigated using Ti-SBA15-CN under visible-light irradiation. By introducing Ti into the SBA-15 framework structure, the visible light driven photocatalytic activity of the obtained Ti-SBA15-CN was higher than SBA15-CN and the photocatalytic activity exhibited a rise with the increase of Ti contents. It was because the presence of Ti moiety could promote the separation of the photo-generated charge carriers in carbon nitride, leading to the enhancement of the photocatalytic activity. The addition of phenol further enhanced the photocatalytic reduction of Cr (VI). Similarly, the presence of Cr (VI) promoted the degradation of phenol. The synergistic effect between the reduction of Cr (VI) and the degradation of phenol provided salutary method for purification of the complex waste water and environmental restoration.
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