钙钛矿(结构)
卤化物
背景(考古学)
纳米技术
材料科学
离子键合
X射线探测器
探测器
带隙
计算机科学
工程物理
光电子学
物理
化学
地质学
电信
化学工程
离子
无机化学
工程类
古生物学
量子力学
作者
Nasir Ali,Khurram Shehzad,Sanam Attique,Amjad Ali,Fazli Akram,Adnan Younis,Shahid Ali,Yun Sun,Guolin Yu,Huizhen Wu,Ning Dai
出处
期刊:Small
[Wiley]
日期:2024-01-17
标识
DOI:10.1002/smll.202310946
摘要
Abstract Owing to their extraordinary photophysical properties, organometal halide perovskites are emerging as a new material class for X‐ray detection. However, the existence of toxic lead makes their commercialization questionable and should readily be replaced. Accordingly, several lead alternatives have been introduced into the framework of conventional perovskites, resulting in various new perovskite dimensionalities. Among these, Pb‐free lower dimensional perovskites (LPVKs) not only show promising X‐ray detecting properties due to their higher ionic migration energy, wider and tunable energy bandgap, smaller dark currents, and structural versatility but also exhibit extended environmental stability. Herein, first, the structural organization of the PVKs (including LPVKs) is summarized. In the context of X‐ray detectors (XDs), the outstanding properties of the LPVKs and active layer synthesis routes are elaborated afterward. Subsequently, their applications in direct XDs are extensively discussed and the device performance, in terms of the synthesis method, device architecture, active layer size, figure of merits, and device stability are tabulated. Finally, the review is concluded with an in‐depth outlook, thoroughly exploring the present challenges to LPVKs XDs, proposing innovative solutions, and future directions. This review provides valuable insights into optimizing non‐toxic Pb‐free perovskite XDs, paving the way for future advancements in the field.
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