离子液体
环境友好型
纳米技术
氢键
化学物理
材料科学
领域(数学)
生化工程
计算机科学
工程物理
化学
物理
分子
有机化学
工程类
催化作用
生态学
数学
纯数学
生物
作者
Yanlei Wang,Hongyan He,Chenlu Wang,Yumiao Lu,Kun Dong,Feng Huo,Suojiang Zhang
出处
期刊:JACS Au
[American Chemical Society]
日期:2022-02-01
卷期号:2 (3): 543-561
被引量:31
标识
DOI:10.1021/jacsau.1c00538
摘要
Ionic liquids (ILs) hold great promise in the fields of green chemistry, environmental science, and sustainable technology due to their unique properties, such as a tailorable structure, the various types available, and their environmentally friendly features. On the basis of multiscale simulations and experimental characterizations, two unique features of ILs are as follows: (1) strong coupling interactions between the electrostatic forces and hydrogen bonds, namely in the Z-bond, and (2) the unique semiordered structure and properties of ultrathin films, specifically regarding the quasi-liquid. In accordance with the aforementioned theoretical findings, many cutting-edge applications have been proposed: for example, CO2 capture and conversion, biomass conversion and utilization, and energy storage materials. Although substantial progress has been made recently in the field of ILs, considerable challenges remain in understanding the nature of and devising applications for ILs, especially in terms of e.g. in situ/real-time observation and highly precise multiscale simulations of the Z-bond and quasi-liquid. In this Perspective, we review recent developments and challenges for the IL research community and provide insights into the nature and function of ILs, which will facilitate future applications.
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