反铁磁性
凝聚态物理
磁化
各向异性
相图
磁各向异性
物理
磁场
相(物质)
量子力学
作者
J. Werner,Changhyun Koo,R. Klingeler,A. N. Vasiliev,E. A. Ovchenkov,Anastasia Polovkova,Grigory V. Raganyan,E.A. Zvereva
出处
期刊:Physical review
[American Physical Society]
日期:2016-09-06
卷期号:94 (10)
被引量:16
标识
DOI:10.1103/physrevb.94.104408
摘要
The magnetic phase diagram and low-energy magnon excitations of structurally\nand magnetically chiral MnSb2O6 are reported. The specific heat and the static\nmagnetization are investigated in magnetic fields up to 9 and 30 T,\nrespectively, while the dynamicmagnetic properties are probed by X-band as well\nas tunable high-frequency electron spin-resonance spectroscopy. Below TN = 11.5\nK, we observe antiferromagnetic resonance modes which imply small but finite\nplanar anisotropy showing up in a zero-field splitting of 20 GHz. The data are\nwell described by means of an easy-plane two-sublattice model with the\nanisotropy field BA = 0.02 T. The exchange field BE = 13 T is obtained from the\nsaturation field derived from the pulsed-field magnetization. A crucial role of\nthe small anisotropy for the spin structure is reflected by competing\nantiferromagnetic phases appearing, at T = 2 K, in small magnetic fields at BC1\n$\\approx$ 0.5 T and BC2 = 0.9 T. We discuss the results in terms of spin\nreorientation and of small magnetic fields favoring helical spin structure over\nthe cycloidal ground state which, at B = 0, is stabilized by the planar\nanisotropy. Above TN, short-range magnetic correlations up to >=60 K and\nmagnetic entropy changes well above TN reflect the frustrated triangular\narrangement of Mn2+ ions in MnSb2O6.\n
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