摩擦电效应
材料科学
纳米技术
纳米发生器
兴奋剂
介孔材料
电极
镱
锐钛矿
分离器(采油)
光电子学
化学工程
光催化
复合材料
催化作用
物理化学
工程类
物理
压电
化学
热力学
生物化学
作者
Manmatha Mahato,Jong‐Nam Kim,Rassoul Tabassian,Araz Rajabi‐Abhari,Ji‐Seok Kim,Sang-Hee Nam,Hyunjoon Yoo,Il‐Kwon Oh
出处
期刊:Nano Energy
[Elsevier]
日期:2021-12-01
卷期号:90: 106615-106615
被引量:10
标识
DOI:10.1016/j.nanoen.2021.106615
摘要
Herein, we report a mutually exclusive ytterbium and nitrogen co-doping strategy for mesoporous titania-carbon (YbNTiO2@C) specially designed for the positive electrode materials towards self-cleaning functionality and high-power triboelectric nanogenerators. Nano-porous structures of YbNTiO2@C having higher surface energy not only provide the enlarge platform for atom-to-atom contacts, but also increase the charge density of the tribo-layer by accelerating the effective electronic quantum transition effects in-between the opposite electrodes in comparison with pristine TiO2. The formation of crystal defects due to doping of ytterbium on the regular lattice structure of TiO2 along with unique substitutional and interstitial nitrogen-doping boosts the overall surface polarity and increases the charge storage and discharge capability when exposed as an interactive electrode surface in dry-type capacitive triboelectric nanogenerators (TENGs). Therefore, YbNTiO2@C coated tribo-positive electrode not only shows considerable enhancement of TENG performances, but also provides significant improvement in self-cleaning function under sunlight. The YbNTiO2@C layer shows remarkable output triboelectricity up to 3 folds and self-cleaning decomposition of methylene blue up to 96.40% within a minute. Notable improvements in both self-cleaning ability and high-performance power generation enable the realization of an ideal smart roof for harvesting green energy from rain and wind in cloud weather.
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