Giant spin Hall angle in the Heusler alloy Weyl ferromagnet Co2MnGa

Weyl semimetals are playing a major role in condensed-matter physics due to exotic topological properties, and their coexistence with ferromagnetism may lead to enhanced spin-related phenomena. Here, the inverse spin Hall effect (ISHE) in the ferromagnetic Weyl semimetal Heusler alloy ${\mathrm{Co}}_{2}\mathrm{MnGa}$ was investigated at room temperature by means of electrical spin injection in lateral spin valve structures. Spin transport properties such as spin polarization and spin diffusion length in this material were precisely extracted in order to estimate the spin Hall angle ${\ensuremath{\theta}}_{\text{SH}}$, which was found to be $\ensuremath{-}0.19\ifmmode\pm\else\textpm\fi{}0.04$ and is among the highest reported for a ferromagnet. Although this value is on the same order of magnitude of known heavy metals, the significantly higher resistivity of ${\mathrm{Co}}_{2}\mathrm{MnGa}$ implies an improvement on the magnitude of detection voltages, while its ferromagnetic nature allows controlling the intensity of SHE through the magnetization direction. It was also shown that Onsager's reciprocity does not hold for this system, which is in part attributable to a different spin-dependent Hall conductivity for spin-up and spin-down carriers.