聚偏氟乙烯
吸附
结垢
化学工程
膜
光催化
过滤(数学)
膜污染
废水
化学
色谱法
材料科学
催化作用
有机化学
废物管理
生物化学
统计
数学
工程类
作者
Liang Zhou,Guoqing Xiao,Yi He,Jingcheng Wu,Heng Shi,Xiangying Yin,Teng He,Zhenyu Li,Jingyu Chen
标识
DOI:10.1016/j.colsurfa.2022.128733
摘要
Multi-functional filtration membranes, with effective purification capacity against diverse emulsified-oils, high adsorption ability for soluble organic dyes in aquatic system, good physical/chemical stability, and strong Photocatalysis induced anti oil/dye fouling functions, are highly desirable for the complex oily sewage purification, but still a challenge to be realized. Herein, a ternary beta-iron oxyhydroxide (β-FeOOH)/halloysite-nanotubes (HNTs)/polyvinylidene fluoride (PVDF) porous membrane has been designed to address this challenge. The resultant membrane exhibits effective separation efficiency towards various oil-water emulsions and high soluble pollutants adsorption by filtration during the rapid oily wastewater purification. Interestingly, it also displays high flux (~6500 L∙m−2∙h−1), good cycling stability (after 5 cycles the flux recovery rate is still closed to 100%), and strong chemical/physical stability. Given the robust photo-Fenton catalytic activity of β-FeOOH, the permeation flux and adsorption capacity of the fouled membrane could be quickly restored (recovery: higher than 99%) within 10 min under visible light irradiation. Our results open an alternative and effective route to solve the oil/dye fouling issue for complex wastewater remedy.
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