高次谐波产生
物理
阿秒
极化(电化学)
激光器
谐波
线极化
圆极化
电子
原子物理学
椭圆极化
电离
对称(几何)
光学
量子力学
磁场
超短脉冲
化学
物理化学
电压
几何学
离子
数学
作者
Kai‐Jun Yuan,André D. Bandrauk
出处
期刊:Physical review
[American Physical Society]
日期:2018-02-07
卷期号:97 (2)
被引量:46
标识
DOI:10.1103/physreva.97.023408
摘要
We present symmetry effects of laser fields and molecular geometries in circularly polarized high-order harmonic generation by bichromatic counter-rotating circularly polarized laser pulses. Simulations are performed on oriented molecules by numerically solving time-dependent Schr\"odinger equations. We discuss how electron recollision trajectories by the orthogonal laser field polarizations influence the harmonic polarization by using a time-frequency analysis of harmonics. It is found that orientation-dependent asymmetric ionization in linear molecules due to Coulomb potentials gives rise to a dependence of the polarization on the harmonic frequency. Effects of Coriolis forces are also presented on harmonic generation. Electron recollision trajectories illustrate the effects of the relative symmetry of the field and the molecule, thus paving a method for circularly polarized attosecond pulse generation and molecular orbital imaging in more complex systems.
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