等离子体
燃烧
氨
氮氧化物
化学
氢
分析化学(期刊)
预混火焰
傅里叶变换红外光谱
等离子体稳定性
材料科学
燃烧室
化学工程
环境化学
物理
有机化学
量子力学
工程类
托卡马克
作者
Rongyuan Ju,Jinhua Wang,Meng Zhang,Haibao Mu,Guanjun Zhang,Jinlu Yu,Zuohua Huang
出处
期刊:Energy
[Elsevier BV]
日期:2023-04-26
卷期号:277: 127649-127649
被引量:47
标识
DOI:10.1016/j.energy.2023.127649
摘要
Ammonia received increased attention as a carbon-free fuel and hydrogen carrier. Poor combustion stability and high NOx emission are the main issues for ammonia combustion. Effects of rotating gliding arc (RGA) discharge plasma on the flame stability and NOx emission of NH3/air premixed swirling flames were investigated. The discharge characteristics of the RGA were studied. The flame stabilization mechanisms by plasma were revealed and analyzed according to the flame structure transition and the distribution of key intermediate OH radicals. The NOx emissions were measured by the Gasmet DX4000 Fourier Transform Infrared (FTIR) gas analyzer. Results showed that the RGA discharge plasma can enhance the stability and extend the lean blow-off (LBO) limits from 0.6 to approximately 0.43–0.57. A hysteresis phenomenon about the transition between the lift-off flame and the attached flame was observed without plasma and disappeared with plasma activation. The plasma reduces NO and NO2 emissions mainly due to the kinetic and cracking effects of plasma. Extremely low NO emission below 300 ppm can be observed for very lean ammonia flames with an equivalence ratio (φ) lower than 0.6, which are stabilized by plasma, while a large amount of unburned NH3 emission is accompanied.
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