High‐Performance Multipedal Shape Strain Sensors for Human Motion and Electrophysiological Signal Monitoring

Abstract Strain sensors from conducting polymer hydrogel have been widely employed in various wearable devices, electronic skins, and biomedical applications. These sensors provide outstanding flexibility and high sensitivity by integrating conducting polymer with hydrogels, making them particularly suitable for monitoring human motion and physiological signals like heart rate or muscle activity. Despite their extensive application potential, conducting polymer hydrogel face several technical challenges in practical use, including poor mechanical properties, lack of long‐term stability, and difficulty in customizable design. This work introduces a method for fabricating a multipedal strain sensor using poly(3,4‐ethylenedioxythiophene):polystyrene sulfonate (PEDOT:PSS)/polyvinyl alcohol (PVA) dimethyl sulfoxide (DMSO)hydrogels through screen printing and demonstrates its application in human motion monitoring. The multipedal strain sensor demonstrates a low Young's modulus (200 kPa), high stretchability (400%), and excellent mechanical cyclic stability (3000 cycles). Furthermore, this strain sensor is further applied to detect human movements such as chewing, smiling, fist clenching, arm bending, and carotid pulse monitoring. Comparative analysis between the multipedal‐designed sensor and the non‐designed sensor highlights the enhanced sensing capabilities of the multipedal sensor. The design of this multipedal sensor holds the potential to broaden the design concepts for strain sensors and offers new insights for wearable devices and electronic skins.