Anisotropic Piezoresistive Sensors Made with Magnetically Induced Vertically Aligned Carbon Nanotubes/Polydimethylsiloxane

A piezoresistive material consisting of internal vertically aligned carbon nanotubes acting in concert with an external microdome structure is prepared to obtain a flexible piezoresistive sensor with high anisotropy. Here, we first obtained flexible piezoresistive composites (VCP) with anisotropic properties by inducing the vertical alignment of multiwalled carbon nanotubes in the pressure direction under a weak magnetic field of 0.6 T. Then, the composite with a microdome structure on the surface (m-VCP) was fabricated by a mold with a microstructure to further increase the anisotropy of the composite. The m-VCP microstructure was docked with VCP and placed between two layers of copper foil. With the synergistic effect of vertically aligned carbon nanotubes and the microdome structure, the sensitivity of the flexible sensor in the pressure direction was dramatically increased. In the low-strain range (0-6%), the sensitivity of m-VCP (GF = 9.208) is improved by 49% compared to m-CP and by 86% compared to VCP. The sensor has high anisotropy in the piezoresistive direction and retains good fatigue resistance under fatigue testing for 2000 cycles. This means that the sensor can be used in emerging fields such as human health monitoring, wearable electronics, and intelligent human-computer interaction.