Voronoi‐Tessellated Graphite Produced by Low‐Temperature Catalytic Graphitization from Renewable Resources

Abstract A highly crystalline graphite powder was prepared from the low temperature (800–1000 °C) graphitization of renewable hard carbon precursors using a magnesium catalyst. The resulting graphite particles are composed of Voronoi‐tessellated regions comprising irregular sheets; each Voronoi‐tessellated region having a small “seed” particle located near their centroid on the surface. This suggests nucleated outward growth of graphitic carbon, which has not been previously observed. Each seed particle consists of a spheroidal graphite shell on the inside of which hexagonal graphite platelets are perpendicularly affixed. This results in a unique high surface area graphite with a high degree of graphitization that is made with renewable feedstocks at temperatures far below that conventionally used for artificial graphites.