环境科学
臭氧
大气科学
灵敏度(控制系统)
气候学
沉积(地质)
臭氧消耗
气候变化
气候敏感性
吨
气候模式
气象学
地面气温
全球变暖
大气(单位)
臭氧层
大气化学
空气污染
对流层臭氧
中国
中国
震级(天文学)
大气模式
全球变化
公制(单位)
标识
DOI:10.1021/acs.est.6c04659
摘要
Abstract Ozone-temperature sensitivity measures the increase in ozone concentration per Kelvin rise in temperature, serving as a critical metric for assessing ozone responses to climate warming. Here, from extensive observations across the Northern Hemisphere, we show that China exhibits a remarkably higher present-day (2017–2024) summertime surface ozone-temperature sensitivity (mΔO3-ΔTmax; 3.7 ppbv K–1) compared to the US (1.6 ppbv K–1) and Europe (1.8 ppbv K–1), with extremely high values reaching 8–10 ppbv K–1 at the site level. GEOS-Chem model simulations with improved accuracy in reproducing observed mΔO3-ΔTmax attribute this elevated sensitivity predominantly to temperature-indirect effects (66%), comprising comparable contributions from temperature-associated changes in radiation (44%) and transport patterns (51%). These indirect effects dominate the spatial and interannual variability of mΔO3-ΔTmax in China. Direct temperature effects on emissions, chemistry, and deposition account for the remaining 34%. Global models project that stringent emission reductions will decrease China’s future mΔO3-ΔTmax to levels comparable to those of the US and Europe, highlighting emission levels as the primary determinant of the magnitude of ozone-temperature sensitivity. These findings emphasize that sustained emission controls are crucial for mitigating the risks associated with compound heat and ozone pollution.
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