钙钛矿(结构)
材料科学
能量转换效率
三碘化物
太阳能电池
钙钛矿太阳能电池
光电子学
开路电压
短路
电流密度
锡
铝
氧化铟锡
兴奋剂
图层(电子)
电极
电压
纳米技术
冶金
电气工程
化学
色素敏化染料
结晶学
物理
物理化学
量子力学
电解质
工程类
作者
Muhammed O. Abdulmalik,Eli Danladi,Rita C. Obasi,P.M. Gyuk,Francis U. Salifu,Suleiman Magaji,Anselem C. Egbugha,Daniel Thomas
标识
DOI:10.26565/2312-4334-2022-4-12
摘要
The toxic lead component as well as the expensive and less stable spiro-OMeTAD in perovskite solar cells (PSCs) pose a great deal of hindrance to their commercial viability. Herein, a computational approach towards modeling and simulation of all inorganic cesium tin-germanium triiodide (CsSnGeI3) based perovskite solar cell was proposed and implemented using solar cell capacitance simulator (SCAPS–1D) tool. Aluminium doped zinc oxide (ZnO:Al) and Copper Iodide (CuI) were used as electron and hole transport layers (ETL and HTL) respectively. The initial device without any optimization gave a power conversion efficiency (PCE) of 24.826%, fill factor (FF) of 86.336%, short circuit current density (Jsc) of 26.174 mA/cm2 and open circuit voltage (Voc) of 1.099 V. On varying the aforementioned parameters individually while keeping others constant, the optimal values are 1000 nm for absorber thickness, 1014 cm-3 for absorber layer defect density, 50 nm for ETL thickness, 1017 cm-3 for ETL doping concentration and 260 K for temperature. Simulating with these optimized values results to PCE of 25.459%, Voc of 1.145 V, Jsc of 25.241 mA/cm2, and a FF of 88.060%. These results indicate that the CsSnGeI3 is a viable alternative absorbing layer for usage in the design of a high PCE perovskite solar cell device.
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