材料科学
光电探测器
碳纳米管
响应度
紫外线
异质结
光电子学
光电效应
纳米管
纳米结构
纳米技术
带隙
半导体
作者
Na Wang,Renrong Zheng,Chen Jiang,Zan Ding,Haisheng San,Shaoda Zhang
标识
DOI:10.1016/j.jsamd.2022.100452
摘要
Self-driven ultraviolet photodetectors based on wide-bandgap semiconductors have been well investigated but are still being explored for further performance enhancement. Here we report a self-driven electrochemical ultraviolet photodetector (EUVPD) using a three-dimensional nanostructured photoanode based on defect-engineered TiO2 nanotube arrays (TNAs) modified with single-walled carbon nanotubes (SWCNTs) to enhance photoelectric performance. The EUVPDs based on Ar-annealed TNAs modified with 0.1 mg/mL of SWCNTs were found to have higher responsivity (∼60 mA/W), higher on/off current ratio (∼4.3 × 103), the faster response time (4 ms of rise-time and 27 ms of decay-time) when compared with unmodified and air-annealed ones. This performance enhancement is attributed to the highly efficient separation and transport of photoexcited carriers through the electrochemical redox reaction in the SWCNTs network anchored on the defect-engineered TNAs/electrolyte heterojunction nanostructure.
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