激光阈值
材料科学
钙钛矿(结构)
可控性
光电子学
激光器
极化(电化学)
谐振器
纳米技术
光学
物理
结晶学
物理化学
波长
化学
数学
应用数学
作者
Yuhan Wang,Yubin Fan,Xudong Zhang,Haijun Tang,Qinghai Song,Jiecai Han,Shumin Xiao
出处
期刊:ACS Nano
[American Chemical Society]
日期:2021-03-17
卷期号:15 (4): 7386-7391
被引量:96
标识
DOI:10.1021/acsnano.1c00673
摘要
Lead halide perovskites have been promising materials for lasing applications. Despite that a series of perovskite microlasers have been reported, their lasing modes are confined by either the as-grown morphology or the etched boundary. The first one is quite random and incompatible with integration, whereas the latter one strongly spoils the laser performances. Herein, we propose and experimentally demonstrate a robust and generic mechanism to realize well-controlled perovskite microlasers without the etching process. By patterning a one-dimensional polymer grating onto a perovskite film, we show that the symmetry-protected bound states in the continuum (BICs) can be formed in it. The intriguing properties of BICs including a widely spread mode profile and high Q factor, associated with the exceptional gain of perovskite, produce single-mode microlasers with high repeatability, controllability, directionality, and a polarization vortex. This mechanism can also be extended to two-dimensional nanostructures, enabling BIC lasers with different topological charges.
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