Full‐Span Reversible Space‐Time Birefringence

ABSTRACT Birefringence, the polarization‐dependent splitting of light in anisotropic crystals, enables diverse optical phenomena and advanced functionalities such as optical communication, nonlinear optics, and quantum optics. However, conventional methods for controlling birefringence typically rely on engineering the optical crystal structure or applying external stimuli such as electric fields, mechanical stress, or thermal variations, which are often constrained by limited tunability, challenges in integration with compact photonic devices, or slow response time. Here, we introduce a new degree of freedom to manipulate the birefringence of light propagation in optical crystals through programming the spatiotemporal spectral phase of the incident light wave. We demonstrate that this approach achieves continuous tuning of birefringence across a spectrum more than 100 times broader than that achievable with conventional birefringence tuning, spanning from positive through zero to negative values, irrespective of the crystal's optical sign and without inherent physical limitations. This unique optical behavior provides a versatile platform for investigating the complex dynamics of wave flow in anisotropic media, while the broad tunability of this space‐time birefringence will spur innovations in ultrafast optical manipulation, optical computation, and quantum information processing—applications that demand rapid and flexible device reconfiguration.