光催化
扫描电子显微镜
降级(电信)
纳米棒
材料科学
钒酸盐
复合数
透射电子显微镜
氮化碳
催化作用
核化学
可见光谱
热液循环
化学工程
复合材料
化学
纳米技术
冶金
有机化学
工程类
光电子学
计算机科学
电信
作者
Danyao Chen,Bolin Liu,Qianmin Pu,Xi Chen,Guangrui Wen,Ze-Sheng Li
标识
DOI:10.1016/j.jhazmat.2019.03.090
摘要
The degradation of tetracycline by silver vanadate (AgVO3), graphite-like carbon nitride (g-C3N4) and their composites was studied by visible light photocatalysis. Their structures and morphologies were studied by X-ray diffraction (XRD), scanning electron microscopy (SEM) and transmission electron microscopy (TEM). Their degradation intermediates were analyzed by GC–MS. Nanorod silver vanadate was synthesized by hydrothermal method. The results show that the gap between nanorods is reduced by adding spinning carbon nitride, and the photocatalytic performance of the composite is stronger than that of single material. The reaction rate constants of Ag-AgVO3/g-C3N4 composites were 0.0298 min−1, 2.4 and 2.0 times that of g-C3N4 (K=0.0125 min-1) and AgVO3 (K=0.0152 min-1), respectively. At 120 minutes, the degradation rate of the composites reached 83.6%. The degradation of tetracycline was confirmed by GC–MS, and a possible degradation process was proposed.
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