Vertical and Lateral Transport of Particulate Radiocesium off Fukushima

微粒 环境科学 福岛核事故 沉积物 泥沙输移 海床 海底管道 焊剂(冶金) 大气科学 水文学(农业) 海洋学 核电站 地质学 化学 地貌学 岩土工程 物理 有机化学 核物理学
作者
Shigeyoshi Otosaka,Takahiro Nakanishi,Takashi Suzuki,Yuhi Satoh,Hisashi Narita
出处
期刊:Environmental Science & Technology [American Chemical Society]
卷期号:48 (21): 12595-12602 被引量:38
标识
DOI:10.1021/es503736d
摘要

Transport processes of particulate radiocesium were investigated using a sediment trap deployed at about 100 km east of the Fukushima Daiichi Nuclear Power Plant. A sediment trap was installed at 873 m depth of the station (119 m above the bottom), and time-series sampling of sinking particles was carried out from August, 2011 to June, 2013. The accident-derived radiocesium was detected from sinking particles over two years after the accident. Observed 137Cs flux was highest in September 2011 (98 mBq m(-2) day(-1): decay-corrected to March 11, 2011), and decreased over time with seasonal fluctuations. Particulate fluxes of radiocesium were mainly affected by two principal processes. One was the rapid sinking of radiocesium-bound particles (moderate mode). This mode was dominant especially in the early postaccident stage, and was presumed to establish the distribution of radiocesium in the offshore seabed. Another mode was observed in winter, and secondary transport of particles attributed to turbulence near the seabed increased fluxes of particulate radiocesium (turbulence mode). Although the latter process would not drastically change the distribution of sedimentary radiocesium in the short term, attention should be paid as this key process redistributing the accident-derived radiocesium may cumulatively affect the long-term distribution.
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