CNT-based gel-coated cotton fabrics for constructing symmetrical evaporator with up/down inversion property for efficient continuous solar desalination

海水淡化 结晶 蒸发器 蒸发 材料科学 聚苯乙烯 太阳能淡化 化学工程 复合材料 化学 热力学 聚合物 工程类 物理 热交换器 生物化学
作者
Ruru Meng,Jun Lyu,Liming Zou,Qiuping Zhong,Zixiao Liu,Bo Zhu,Meiyue Chen,Lisha Zhang,Zhigang Chen
出处
期刊:Desalination [Elsevier BV]
卷期号:554: 116494-116494 被引量:17
标识
DOI:10.1016/j.desal.2023.116494
摘要

Solar-driven seawater desalination has drawn much attention, while the practical application has been limited by the unsatisfactory photoabsorption as well as solid-salt crystallization. To address the issues, hereby we have constructed a symmetrical evaporator with up/down inversion property by using carbon nanotubes (CNTs)-based gel-coated cotton fabrics. Such CNT-cotton fabrics have porous structure and strong photoabsorption in 280–2500 nm range. Subsequently, two CNT-cotton fabrics are coated on cotton-embedded polystyrene for constructing symmetrical evaporator. Such symmetrical evaporator is placed in NaCl solution (3.5 wt%), it exhibits an excellent evaporation rate of 1.62 kg m−2 h−1 under 1 sun irradiation. To investigate the effects of solid-salt crystallization, a higher concentration of NaCl solution (21 wt%) can be used for evaporation. As expected, the evaporation rate decreases from 1.62 to 0.75 kg m−2 h−1 in 8 h because of solid-salt crystallization on the upper-surface. Importantly, the symmetrical evaporator can eliminate adverse effect of solid-salt crystallization by using an inverse strategy (twice an hour), remaining a stable evaporation rate (1.49–1.62 kg m−2 h−1) during long-time test. Therefore, the present design of CNT-cotton fabrics and symmetrical evaporator may provide some new insights for efficient continuous desalination under sunlight irradiation.
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