纳米片
污染物
环境友好型
吸附
环境科学
水污染物
环境化学
环境工程
水处理
水污染
废物管理
环境保护
化学
工程类
生态学
化学工程
生物
有机化学
作者
Xingguo Cai,Jianming He,Liang Chen,Kai Chen,Yulian Li,Kaisheng Zhang,Zhen Jin,Jinyun Liu,Chengming Wang,Xuguang Wang,Lingtao Kong,Jinhuai Liu
出处
期刊:Chemosphere
[Elsevier]
日期:2017-03-01
卷期号:171: 192-201
被引量:125
标识
DOI:10.1016/j.chemosphere.2016.12.073
摘要
A novel graphitic carbon nitride (g-C3N4) nanosheet adsorbent with a large surface area, remarkable hydrophilicity and high adsorption capacity, was presented for the removal of cadmium ions (Cd2+) and methylene blue (MB) from aqueous solution. Adsorption measurements were conducted systematically to study the influences of the contact time, initial concentrations of Cd2+ and MB, temperature, and pH value. The maximum adsorption capacities of g-C3N4 towards Cd2+ and MB were 94.4 and 42.1 mg g-1, respectively, at 318.5 K when the initial concentrations of Cd2+ and MB were 200 and 20 mg L-1, respectively. The adsorption kinetics fit a pseudo-second-order model. The high adsorption performance of the g-C3N4 adsorbent can be attributed to the multiple adsorption sites on g-C3N4, including the π-π conjugate interactions and electrostatic attractions with pollutants in water. In addition, it is significant to achieve high adsorption performance of g-C3N4 nanosheets by efficiently exposing the adsorption sites by adjusting the microstructure surface properties and dispersity in solution.
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